Surface electronic properties of polycrystalline bulk and thin film In2O3(ZnO)k compounds
Identifieur interne : 000437 ( Main/Repository ); précédent : 000436; suivant : 000438Surface electronic properties of polycrystalline bulk and thin film In2O3(ZnO)k compounds
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Abstract
The surface electronic potentials of In2O3(ZnO)k compounds were measured by X-ray and ultraviolet photoelectron spectroscopy. Both thin film (k=2) and bulk specimens (k=3, 5, 7, 9) were studied. All bulk specimens exhibited In enrichment at the surface. All samples showed an increase of In core level binding energies compared to pure and Sn-doped In2O3. The work functions and Fermi levels spanned a range similar to those of the basis oxides In2O3 and ZnO, and the ionization potential was similar to that of both In2O3 and ZnO processed under similar conditions (7.7 eV). This ionization potential was independent of both composition and post-deposition oxidation and reduction treatments. Kelvin probe measurements of cleaned and UV-ozone treated specimens under ambient conditions were in agreement with the photoelectron spectroscopy measurements.
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Surface electronic properties of polycrystalline bulk and thin film In<sub>2</sub>
O<sub>3</sub>
(ZnO)<sub>k</sub>
compounds</title>
<author><name sortKey="Mitchell Hopper, E" uniqKey="Mitchell Hopper E">E. Mitchell Hopper</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Materials Science & Engineering, Northwestern University</s1>
<s2>Evanston, IL 60208</s2>
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<country>États-Unis</country>
<wicri:noRegion>Evanston, IL 60208</wicri:noRegion>
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</author>
<author><name>QIMIN ZHU</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Materials Science & Engineering, Northwestern University</s1>
<s2>Evanston, IL 60208</s2>
<s3>USA</s3>
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<country>États-Unis</country>
<wicri:noRegion>Evanston, IL 60208</wicri:noRegion>
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<author><name sortKey="Gassmann, J Rgen" uniqKey="Gassmann J">J Rgen Gassmann</name>
<affiliation wicri:level="3"><inist:fA14 i1="02"><s1>Institute of Materials Science, Darmstadt University of Technology</s1>
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<author><name sortKey="Klein, Andreas" uniqKey="Klein A">Andreas Klein</name>
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</author>
<author><name sortKey="Mason, Thomas O" uniqKey="Mason T">Thomas O. Mason</name>
<affiliation wicri:level="1"><inist:fA14 i1="01"><s1>Department of Materials Science & Engineering, Northwestern University</s1>
<s2>Evanston, IL 60208</s2>
<s3>USA</s3>
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<country>États-Unis</country>
<wicri:noRegion>Evanston, IL 60208</wicri:noRegion>
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<title level="j" type="abbreviated">Appl. surf. sci.</title>
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<profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Indium</term>
<term>Inorganic compounds</term>
<term>Ionization potential</term>
<term>Kelvin probe</term>
<term>Photoelectron spectroscopy</term>
<term>Surface properties</term>
<term>Thin films</term>
<term>Transition element compounds</term>
<term>Work functions</term>
<term>Zinc oxide</term>
</keywords>
<keywords scheme="Pascal" xml:lang="fr"><term>Propriété surface</term>
<term>Couche mince</term>
<term>Indium</term>
<term>Spectrométrie photoélectron</term>
<term>Sonde Kelvin</term>
<term>Potentiel ionisation</term>
<term>Travail sortie</term>
<term>Oxyde de zinc</term>
<term>O Zn</term>
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<front><div type="abstract" xml:lang="en">The surface electronic potentials of In<sub>2</sub>
O<sub>3</sub>
(ZnO)<sub>k</sub>
compounds were measured by X-ray and ultraviolet photoelectron spectroscopy. Both thin film (k=2) and bulk specimens (k<sub>=</sub>
3, 5, 7, 9) were studied. All bulk specimens exhibited In enrichment at the surface. All samples showed an increase of In core level binding energies compared to pure and Sn-doped In<sub>2</sub>
O<sub>3</sub>
. The work functions and Fermi levels spanned a range similar to those of the basis oxides In<sub>2</sub>
O<sub>3</sub>
and ZnO, and the ionization potential was similar to that of both In<sub>2</sub>
O<sub>3</sub>
and ZnO processed under similar conditions (7.7 eV). This ionization potential was independent of both composition and post-deposition oxidation and reduction treatments. Kelvin probe measurements of cleaned and UV-ozone treated specimens under ambient conditions were in agreement with the photoelectron spectroscopy measurements.</div>
</front>
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O<sub>3</sub>
(ZnO)<sub>k</sub>
compounds</s1>
</fA08>
<fA11 i1="01" i2="1"><s1>MITCHELL HOPPER (E.)</s1>
</fA11>
<fA11 i1="02" i2="1"><s1>QIMIN ZHU</s1>
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<fA11 i1="03" i2="1"><s1>GASSMANN (Jürgen)</s1>
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<fA11 i1="04" i2="1"><s1>KLEIN (Andreas)</s1>
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<fA11 i1="05" i2="1"><s1>MASON (Thomas O.)</s1>
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<fA14 i1="01"><s1>Department of Materials Science & Engineering, Northwestern University</s1>
<s2>Evanston, IL 60208</s2>
<s3>USA</s3>
<sZ>1 aut.</sZ>
<sZ>2 aut.</sZ>
<sZ>5 aut.</sZ>
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<fA14 i1="02"><s1>Institute of Materials Science, Darmstadt University of Technology</s1>
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<fC01 i1="01" l="ENG"><s0>The surface electronic potentials of In<sub>2</sub>
O<sub>3</sub>
(ZnO)<sub>k</sub>
compounds were measured by X-ray and ultraviolet photoelectron spectroscopy. Both thin film (k=2) and bulk specimens (k<sub>=</sub>
3, 5, 7, 9) were studied. All bulk specimens exhibited In enrichment at the surface. All samples showed an increase of In core level binding energies compared to pure and Sn-doped In<sub>2</sub>
O<sub>3</sub>
. The work functions and Fermi levels spanned a range similar to those of the basis oxides In<sub>2</sub>
O<sub>3</sub>
and ZnO, and the ionization potential was similar to that of both In<sub>2</sub>
O<sub>3</sub>
and ZnO processed under similar conditions (7.7 eV). This ionization potential was independent of both composition and post-deposition oxidation and reduction treatments. Kelvin probe measurements of cleaned and UV-ozone treated specimens under ambient conditions were in agreement with the photoelectron spectroscopy measurements.</s0>
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<s5>06</s5>
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<s4>INC</s4>
<s5>32</s5>
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<s4>INC</s4>
<s5>33</s5>
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<s4>INC</s4>
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